Trump announced on Friday that the US would keep the pact in place and waive sanctions against Iran for the "last time", in order to secure agreement from the US' European allies to fix its "terrible flaws".
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Describing sanctions against Larijani as "hostile action", iran's foreign ministry said the move "crossed all red lines of conduct in the international community and is a violation of international law and will surely be answered by a serious reaction of the Islamic republic", state media reported.
Iranian Foreign Minister Mohammad Javad Zarif called Trump's decision an attempt to "undermine" the deal.
Trump plans to negotiate a separate agreement to address flaws he says exists in the Joint Comprehensive Plan of Action (JCPOA), the official name for the 2015 agreement. French President Emmanuel Macron stressed to Trump in a telephone call on Thursday the importance of abiding by the deal.
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It also said Iran would not allow the deal to be linked to other issues, after Mr Trump suggested that the sanctions relief under the deal be tied to Iran limiting its long-range ballistic missile program. He would negotiate that deal with the UK, France, and Germany - but not with Russia, China, and Iran.
Iran argues that continued US sanctions on non-nuclear areas such as human rights and missile testing have effectively barred Iran from gaining many of the financial benefits expected from the deal. The next deadline for Trump to waive sanctions falls on Friday.
Trump wants the European nations that are signatories to the deal to impose permanent restrictions on Iran's uranium enrichment. Would you rather deal with those things with Iran having nuclear weapons or not having them?
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This would not entail negotiations with Iran but would be the result of talks with European allies, the official said. "Staying in this deal, which is a strong one, is vital to enhancing America's, and the world's, security, and avoiding a nuclear arms race in the Middle East".